Real Madrid will face holders Chelsea in the Champions League quarter-finals, while Manchester City tackle Atletico Madrid.
The clash of 13-time winners Madrid and two-time champions Chelsea will be a repeat of last season's semi-final, which the English side won 3-1 on aggregate, and will mean Los Blancos boss Carlo Ancelotti goes up against his former team.
Madrid's Eden Hazard and Thibaut Courtois could also face their old club, who are in a state of crisis after owner Roman Abramovich was hit with UK government sanctions.
The winners of that standout tie will progress to a semi-final against City or Atletico, who meet in a tantalising clash that will see coaches Pep Guardiola and Diego Simeone at the heart of the narrative.
Atletico beat Manchester United at the last-16 stage and will return to the north-west of England in pursuit of another major scalp.
Villarreal, who sprung a surprise by knocking out Juventus, have been rewarded with a clash against Bayern Munich, who were 8-2 aggregate winners over Salzburg.
Benfica will face Jurgen Klopp's in-form Liverpool. The Reds are six-time European champions but lost to the Portuguese giants at the last-16 stage in the 2005-06 season, their last meeting in the Champions League.
The two-leg quarter-final ties will be played April 5-6 and April 12-13, with the semi-finals scheduled for April 26-27 and May 3-4.
The Stade de France will stage the final on May 28, after St Petersburg was stripped of the match due to Russian military action in Ukraine.
Quarter-final draw
Chelsea v Real Madrid
Manchester City v Atletico Madrid
Villarreal v Bayern Munich
Benfica v Liverpool
Semi-final draw
Manchester City/Atletico Madrid v Chelsea/Real Madrid
Benfica/Liverpool v Villarreal/Bayern Munich
Postecoglou: Spurs have a confidence problem to overcome
Ange Postecoglou says that Tottenham need to "overcome" their low confidence after suffering a 4-2 defeat to Liverpool on Sunday.
Spurs slipped to their fourth consecutive Premier League defeat, being left to bemoan their slow start as they found themselves 4-0 down by the hour mark thanks to goals from Mohamed Salah, Andrew Robertson, Cody Gakpo and Harvey Elliott.
Richarlison came off the bench to salvage some pride for Spurs, scoring one before setting up Son Heung-min for a goal on his 300th Premier League appearance.
Spurs had the opportunity to cut the gap to the top four after Aston Villa’s defeat to Brighton, but they remain seven points off a Champions League spot.
Postecoglou’s side still have a game in hand over the Villans, though he was sure that Spurs would be able to put their recent poor run behind them.
Asked if Spurs had a confidence problem, Postecoglou told Sky Sports: "Maybe in the front third there is.
"It probably is a bit of a lack of confidence, but again, that's something the guys have to work through.
"You have to find a way to overcome that because, ultimately, if you don't put pressure on the opposition in the front third after you've worked your way up there, they're going to get comfortable with their position."
Spurs have won just one of their last nine Premier League away games, failing to win any of the last five.
Despite that run extending at Anfield, Postecoglou highlighted what he thought was an improvement on their recent performances.
He continued: "Obviously a hugely disappointing outcome for us but at least we were more like ourselves today in terms of our football.
"Our last two away games at Newcastle and Chelsea, apart from the results which weren't great either, we just didn't try and play our football.
"I thought today, even in the first half, some of our football, our pressing was back to where it should be."
Klopp hails 'special' Anfield following Tottenham win
Jurgen Klopp says Anfield "was a special place" after Liverpool got back to winning ways at home against Tottenham in the Premier League on Sunday.
The Reds cruised into a 4-0 lead against Spurs by the 59th minute as Mohamed Salah and Harvey Elliott played starring roles, with Andrew Robertson and Cody Gakpo also getting on the scoresheet.
They were set up for a slightly nervous finish by Spurs, with substitute Richarlison coming on to score and assist late on to half the deficit to 4-2 by the final whistle.
Victory kept Liverpool’s very slim title hopes alive after a recent dip in form that saw them take just one win from five before this, and Klopp was pleased with the Reds’ reaction in his penultimate game at Anfield.
"We are outstanding until we are not," the German told Sky Sports. "It was a really good game. Tottenham can put pressure on Aston Villa again for the Champions League. In high-performance things, you need a spark.
"Anfield was a special place today. We were 4-0 up, I made the changes, and we lost organisation. Tottenham showed how good they could be. I was happy with the performance.
"We were good in pretty much all areas offensively. The passes were good. So many things were good. We stayed calm. As long as they don't break the lines, then it's fine. Let them pass. I liked our game a lot. The goals were outstanding.
"You do it when you do it and if you miss it, then you miss it. If we win all three, then we can achieve the fifth-highest points tally of Liverpool.
"I would be lying if I said I was at my highest emotion, but I have another game. In two weeks’ time is another day. I have said it before, I love absolutely everything about this club."
Salah was restored to the starting line-up against Spurs after making headlines last weekend for a spat with Klopp on the sideline before he was brought on as a substitute.
He scored the opening goal for Liverpool and became the first player in Premier League history to score 10+ goals and provide 10+ assists in three consecutive seasons. He is also only the second player to tally 10+ in both in five separate seasons in the competition overall, after Wayne Rooney.
After assuring that the rift between him and Salah was resolved in the build-up to this game, Klopp was quick to praise his star man.
He added: "Mo was outstanding, he played a really good game. His side with Harvey [Elliott] was good. I was pleased for him.
"None of the boys want to play not great, why would they? Mo showed what he is capable of."
Salah makes Premier League history in Anfield thriller
Mohamed Salah made more Premier League history as he scored and provided an assist in Liverpool's 4-2 win over Tottenham.
Salah, who had a public disagreement with outgoing Liverpool boss Jurgen Klopp during last week's 2-2 draw with West Ham, was back at his best as the Reds returned to winning ways on Sunday.
He opened the scoring in the 16th minute at Anfield, where Liverpool cruised into a 4-0 lead before Spurs fought back to make matters interesting late on.
Harvey Elliott curled in Liverpool's fourth goal, having received a pass from Salah, who in the process went into the Premier League's record books.
Salah is the first player in Premier League history to score 10+ goals and provide 10+ assists in three consecutive seasons.
Meanwhile, he is also only the second player to tally 10+ in both in five separate seasons in the competition overall, after Wayne Rooney.
"Mo was absolutely outstanding," Klopp told Sky Sports.
Salah's earlier goal had also seen him draw level with Harry Kane as the highest goalscorer in Premier League matches between Liverpool and Spurs, with nine. He is also squandered a great chance to make it 5-2, before seeing a goal disallowed for offside in stoppage time.
Indeed, the fixture itself is now the highest-scoring one in Premier League history, having overtaken Arsenal v Liverpool.
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